Highly Efficient and Monodisperse Graphene Oxide Furnished Ru/Pd Nanoparticles for the Dehalogenation of Aryl Halides via Ammonia Borane

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dc.contributor.authorGöksu, Haydar
dc.contributor.authorYıldız, Yunus
dc.contributor.authorÇelik, Betül
dc.contributor.authorYazıcı, Melike
dc.contributor.authorKılbaş, Benan
dc.contributor.authorŞen, Fatih
dc.date.accessioned2020-05-01T12:10:22Z
dc.date.available2020-05-01T12:10:22Z
dc.date.issued2016
dc.departmentDÜ, Kaynaşlı Meslek Yüksekokuluen_US
dc.descriptionWOS: 000395396400013en_US
dc.description.abstractHighly monodisperse graphene oxide-supported Ru/Pd nanoparticles (RuPd@GO NPs) have been reproducibly and easily synthesized by microwave assisted method. RuPd@GO NPs was performed for dehalogenation of arylhalides in the presence of ammonia borane in a mild condition as novel, highly efficient and exceptional reusable heterogeneous catalyst. The novel materials were characterized by transmission electron microscopy (TEM), the high resolution electron micrograph (HRTEM), X-ray diffraction (XRD) and X-ray photoelectron spectroscopy (XPS). The results showed that the prepared catalysts are highly crystalline, monodisperse and colloidally stable. The current one-pot catalytic process was described as a new methodology for dehalogenation of arylhalides which can be assessed as a quite simple, eco-friendly and highly efficient as well as exceptional reusable. All products were provided with one of the highest yield and the shortest time in the presence of novel RuPd@GO NPs due to the the synergistic effect of Ru and Pd. Our synthesis process comes with a facile and eco-friendly option to RuPd@GO NPs, allowing further scrutiny of current catalysts for numerous other chemical reactions.en_US
dc.description.sponsorshipDuzce UniversityDuzce University [2013.05.03.188, 2015.26.04.371]; Dumlupinar University Research FundDumlupinar University [2014-05, 2015-35, 2015-50]; Science Academy; FABEDen_US
dc.description.sponsorshipThis research was supported by Duzce University (grant no. 2013.05.03.188 and 2015.26.04.371) and Dumlupinar University Research Fund (2014-05, 2015-35 and 2015-50). The partial supports from Science Academy and FABED are highly acknowledged.en_US
dc.identifier.doi10.1002/slct.201600207en_US
dc.identifier.endpage958en_US
dc.identifier.issn2365-6549
dc.identifier.issue5en_US
dc.identifier.scopusqualityQ2en_US
dc.identifier.startpage953en_US
dc.identifier.urihttps://doi.org/10.1002/slct.201600207
dc.identifier.urihttps://hdl.handle.net/20.500.12684/6167
dc.identifier.volume1en_US
dc.identifier.wosWOS:000395396400013en_US
dc.identifier.wosqualityQ4en_US
dc.indekslendigikaynakWeb of Scienceen_US
dc.indekslendigikaynakScopusen_US
dc.language.isoenen_US
dc.publisherWiley-V C H Verlag Gmbhen_US
dc.relation.ispartofChemistryselecten_US
dc.relation.publicationcategoryMakale - Uluslararası Hakemli Dergi - Kurum Öğretim Elemanıen_US
dc.rightsinfo:eu-repo/semantics/closedAccessen_US
dc.subjectDehalogenationen_US
dc.subjectRuPd@GO NPsen_US
dc.subjectammonia boraneen_US
dc.subjectgraphene oxideen_US
dc.subjectnanoparticlesen_US
dc.titleHighly Efficient and Monodisperse Graphene Oxide Furnished Ru/Pd Nanoparticles for the Dehalogenation of Aryl Halides via Ammonia Boraneen_US
dc.typeArticleen_US

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